Formaldehyde Oxidation of Ce0.8Zr0.2O2 Nanocatalysts for Room Temperature: Kinetics and Effect of pH Value
Yang Z. Qin G. Tang R. Jia L. Wang F. Liu T.
July 2023Multidisciplinary Digital Publishing Institute (MDPI)
Nanomaterials
2023#13Issue 14
Ce0.8Zr0.2O2 catalysts were prepared via the co-precipitation method under different pH conditions. The catalysts were characterized via TEM, XRD, XPS, BET, Raman, and FTIR. The oxidation performance of formaldehyde was tested. Precipitation pH affects the physicochemical properties and performance of the Ce0.8Zr0.2O2 catalyst. By controlling the precipitation pH at 10.5, the Ce0.8Zr0.2O2 catalyst with the largest specific surface area, the smallest grain size with the best formaldehyde removal rate (98.85%), abundant oxygen vacancies, and the best oxidation performance were obtained. Meanwhile, the kinetic parameters of the catalyst were experimentally investigated and the calculated activation energy was 12.6 kJ/mol and the number of reaction steps was 1.4 and 1.2.
catalytic oxidation , Ce0.8Zro.2O2 catalysts , formaldehyde , kinetics parameters
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Department of Chemistry and Chemical Technology, Kh. Dosmukhamedov Atyrau University, Studenchesky Ave., 1, Atyrau, 060011, Kazakhstan
China Energy Engineering Group Yunnan Electric Power Design Institute Co., Ltd, Kunming, 650051, China
Department of Chemistry and Chemical Technology
China Energy Engineering Group Yunnan Electric Power Design Institute Co.
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