Ni-Al Self-Propagating High-Temperature Synthesis Catalysts in Dry Reforming of Methane to Hydrogen-Enriched Fuel Mixtures
Tungatarova S. Xanthopoulou G. Vekinis G. Karanasios K. Baizhumanova T. Zhumabek M. Sadenova M.
October 2022MDPI
Catalysts
2022#12Issue 10
The worldwide increase in demand for environmentally friendly energy has led to the intensification of work on the synthesis of H2-containing fuel. The dry reforming of methane has become one of the most important avenues of research since the consumption of two greenhouse gases reduces the rate of global warming. A study of NiAl composite materials as catalysts for methane reforming has been carried out. Self-propagating high-temperature synthesis (SHS) has been used to produce NiAl catalysts. Comparative studies were carried out regarding the dry reforming and partial oxidation of methane, as well as catalysts prepared using the impregnation (IM) and SHS methods. A catalyst with 29% Ni and 51% Al after SHS contains the phases of NiAl and NiAl2O4, which are active phases in the dry reforming of methane. The optimal crystal lattice parameter (for the maximum possible conversion of CO2 and CH4) is 3.48–3.485 Å for Al2O3, which plays the role of a catalyst carrier, and 1.42 Å, for NiAl2O4, which plays the role of a catalyst. The aim of the work is to develop a new and efficient catalyst for the dry reforming of methane into a synthesis gas, which will further promote the organization of a new era of environmentally friendly energy-saving production methods.
catalyst , dry reforming , methane , partial oxidation , SHS combustion synthesis
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D.V. Sokolsky Institute of Fuel, Catalysis and Electrochemistry, 142, Kunaev Str, Almaty, 050010, Kazakhstan
Department of Chemistry and Chemical Technology, Al-Farabi Kazakh National University, 71, Al-Farabi Str, Almaty, 050040, Kazakhstan
Institute of Nanoscience and Nanotechnology, NCSR Demokritos, Aghia Paraskevi, Athens, 15310, Greece
Priority Department Centre “Veritas”, D. Serikbayev East, Kazakhstan State Technical University, 19, Serikbayev Str, Ust-Kamenogorsk, 070000, Kazakhstan
D.V. Sokolsky Institute of Fuel
Department of Chemistry and Chemical Technology
Institute of Nanoscience and Nanotechnology
Priority Department Centre “Veritas”
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